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Structure and bonding of IrB₁₂⁻: converting a rigid boron B₁₂ platelet to a Wankel motor

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Abstract:

The global minimum of IrB₁₂⁻ is a C₃ᵥ symmetric bowl-like structure in which the Ir atom is located on the concave side of the bowl, similar to its lighter congeners, CoB₁₂⁻ and RhB₁₂⁻ clusters. Although all these MB₁₂⁻ (M = Co, Rh, Ir) clusters show dynamical behaviour, analogous to that of the so-called ‘Wankel motors’, the energy barrier for the rotation of the inner B₃ ring within the peripheral B₉ ring is the lowest in the IrB₁₂⁻ case (5.0 kcal mol⁻¹ only). The geometrical feature along with the lower interaction energy between B₃ and MB₉ moieties are responsible for a smaller rotational energy barrier in IrB₁₂⁻ than those in CoB₁₂⁻ and RhB₁₂⁻ clusters.

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Boron and Carbon Nanomaterials Research

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FuenteRSC Advances
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