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Nonequilibrium optical response of a one-dimensional Mott insulator

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Abstract:

We define, compute, and analyze the nonequilibrium differential optical conductivity of the one-dimensional extended Hubbard model at half-filling after applying a pump pulse, using the time-dependent density matrix renormalization group method. The melting of the Mott insulator is accompanied by a suppression of the local magnetic moment and ensuing photogeneration of doublon-holon pairs. The differential optical conductivity reveals (i) mid-gap states related to parity-forbidden optical states and (ii) strong renormalization and hybridization of the excitonic resonance and the absorption band, yielding a Fano resonance. We offer evidence and interpret such a resonance as a signature of nonequilibrium optical excitations resembling excitonic strings, (bi)excitons, and unbound doublon-holon pairs, depending on the magnitude of the intersite Coulomb repulsion. We discuss our results in the context of pump and probe spectroscopy experiments on organic Mott insulators.

Tópico:

Quantum many-body systems

Citaciones:

Citations: 11
11

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Información de la Fuente:

SCImago Journal & Country Rank
FuentePhysical review. B./Physical review. B
Cuartil año de publicaciónNo disponible
Volumen104
Issue8
Páginas085122 - N/A
pISSNNo disponible
ISSN2469-9969

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