In this paper the spectral-luminescent characteristics and study of laser generation properties of new organic compounds are shown, whose particularity consists of forming excited state complexes that allow laser effect obtention. The intense generation of radiation observed in these excited state complexes allows laser creation by active media working at a broad multi- spectral range (the violet and yellow region of the spectrum). The dye laser performance using these dyes has also been investigated using the solvents ethanol and toluene under nitrogen- laser pumping to compare with the commercially available standard dye POPOP, which generates radiation in the violet spectrum region.